화학공학소재연구정보센터
학회 한국공업화학회
학술대회 2021년 가을 (11/03 ~ 11/05, 대구 엑스코(EXCO))
권호 25권 2호
발표분야 포스터-환경·에너지
제목 N-doped graphene oxide enfolded reduced titania for highly stable and selective gas-phase photocatalytic CO2 reduction into CH4
초록 A desire for renewable alternatives to fossil fuels can be achieved by utilizing CO2, H2O, and solar energy to generate solar fuels. Herein, N-doped graphene oxide enfolded reduced titania (NGO-RT) composite was demonstrated for photocatalytic CO2 reduction into CH4. Further, the Pt NPs were deposited on NGO-RT that increases the catalytic performance towards CH4 formation. The optimized Pt1.0%-NGO-RT catalyst displayed a selective visible-light CO2 reduction into CH4 using a flow reactor system with ≈12 and ≈2 times higher activity than pristine RT and NGO-RT, respectively. The catalyst demonstrated long-term stability over 35 h. The improved catalytic performance can be attributed to RT’s downward band bending at the NGO-RT interface.
저자 Chaitanya B. Hiragond, 인수일
소속 DGIST
키워드 Photocatalysis; CO2 reduction; Gas phase
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