A systematic experimental investigation to determine the shear, tensile, and fracture properties of adhesive joints with bonded same-materials (polymer-polymer) and bi-materials (metal-polymer) is reported. Full-field optical techniques including photoelasticity and coherent gradient sensing (CGS) are employed to record the stress development and failure in these adhesive joints. Five types of strong and weak adhesives are used in conjunction with five different types of materials [aluminum, steel, polymethylmethacrylate (PMMA), polycarbonate, and Homalite (R)-100] to produce a variety of bonded material systems. Weld-on (R)-10 and a polyester bonding consistently show higher tensile and shear bonding strengths. Bi-material systems in shear and fracture report lower properties than the same-material systems due to a higher property mismatch in the former. The resulting complete experimental data are expected to be immensely helpful to computational mechanists in simulating failure mechanics of adhesive joints.