Nature Materials, Vol.12, No.5, 387-391, 2013
Fluctuating charge-density waves in a cuprate superconductor
Cuprate materials hosting high-temperature superconductivity (HTS) also exhibit various forms of charge and spin ordering(1-6) whose significance is not fully understood(7). So far, static charge-density waves(8) (CDWs) have been detected by diffraction probes only at particular doping levels(9-11) or in an applied external field(12). However, dynamic CDWs may also be present more broadly and their detection, characterization and relationship with HTS remain open problems. Here we present a method based on ultrafast spectroscopy to detect the presence and measure the lifetimes of CDW fluctuations in cuprates. In an underdoped La1.9Sr0.1CuO4 film (T-c = 26 K), we observe collective excitations of CDW that persist up to 100 K. This dynamic CDW fluctuates with a characteristic lifetime of 2 ps at T = 5 K that decreases to 0.5 ps at T = 100 K. In contrast, in an optimally doped La1.84Sr0.16CuO4 film (T-c = 38.5 K), we detect no signatures of fluctuating CDWs at any temperature, favouring the competition scenario. This work forges a path for studying fluctuating order parameters in various superconductors and other materials.