화학공학소재연구정보센터
Journal of Industrial and Engineering Chemistry, Vol.20, No.2, 682-688, March, 2014
Preparation of copper containing methacrylic polymers and their application for the copper patterns
E-mail:
Copper containing methacrylic polymers were prepared by the polymerization of a copper methacrylate complex (Cu[CH2=C(CH3)-COO](COD), where COD = 1,5-cyclooctadiene) with different methylmetha-crylate and methacrylic acid compositions. These polymers were found to be soluble in many organic solvents including THF and chloroform. Copper nano-networks or aggregated nanoparticles were obtained when a THF solution of the polymers was reduced using an aqueous sodium borohydride solution. When a thin film of the polymers coated on a silicon wafer was irradiated with an electron beam, nanoparticles were produced on the irradiated area, while the non-irradiated areas could be washed away with a weak base developer, such as a tetramethylammoniumhydroxyde (TMAH) aqueous solution, to produce a copper pattern through an electron beam lithography process.
  1. Daniel MC, Astruc D, Chem. Rev., 104(1), 293 (2004)
  2. Sato M, Shindo H, Kondo K, Takemoto K, J. Polym. Sci. A: Polym. Chem., 18, 101 (1980)
  3. Sun CM, Qu RJ, Sun XR, Ji CN, Wang CH, J. Appl. Polym. Sci., 103(2), 963 (2007)
  4. Marambio OG, Pizarro GD, Jeria-Orell M, Huerta M, Olea-Azar C, Habicher WD, J. Polym. Sci. A: Polym. Chem., 43(20), 4933 (2005)
  5. Calzia KJ, Tew GN, Macromolecules, 35(16), 6090 (2002)
  6. Mathew B, Rajasekharan pillai NR, Eur. Polym, 30, 61 (1994)
  7. Chacko S, Mathew T, Kuriakose S, J. Appl. Polym. Sci., 90(10), 2684 (2003)
  8. Supriya L, Unal S, Long TE, Claus RO, Chem. Mater., 18, 2506 (2006)
  9. Annenkov VV, Danilovtseva EN, Saraev VV, Mikhaleva AI, J. Polym. Sci. A: Polym. Chem., 41(14), 2256 (2003)
  10. Belfiore LA, Mccurdie MP, J. Polym. Sci. B: Polym. Phys., 33(1), 105 (1995)
  11. Akamatsu K, Ikeda S, Nawafune H, Deki S, Chem. Mater., 15, 2488 (2003)
  12. Anyaogu KC, Fedorov AV, Neckers DC, Langmuir, 24(8), 4340 (2008)
  13. Van den hende JH, Baird WC, J. Am. Chem. Soc., 85, 1009 (1963)
  14. Reger DI, Dukes MD, J. Organomet, 113, 173 (1976)
  15. Chi KM, Corbitt TS, Hampeden-Smith MJ, Kodas TT, Duesler EN, J. Organomet, 449, 181 (1993)
  16. Wang SX, Wang MT, Lei Y, Zhang LD, J. Mater. Sci. Lett., 18(24), 2009 (1999)
  17. Tao YT, J. Am. Chem, 115, 4350 (1993)
  18. Okoroanyanwu U, Byers J, Shimokawa T, Willson CG, Chem. Mater., 10, 3328 (1998)
  19. Balke ST, Hamielec AE, J. Appl. Polym. Sci., 17, 905 (1973)
  20. Jarray J, Larbi FBC, Vanhulle F, Dubault A, Halary JL, Macromol. Symp., 198, 103 (2003)
  21. Kuo SW, Wu CH, Chang FC, Macromolecules, 37(1), 192 (2004)
  22. Kaliyappan T, Rajagopan S, Kannan P, J. Appl. Polym. Sci., 90(8), 2083 (2003)
  23. Mansur CRE, Tavares MIB, Monteiro EEC, J. Appl. Polym. Sci., 75(4), 495 (2000)
  24. Dhas NA, Raj CP, Gedanken A, Chem. Mater., 10, 1446 (1998)
  25. Lisiecki I, Pileni MP, J. Phys. Chem., 99(14), 5077 (1995)
  26. Kim JU, Cha SH, Shin K, Jho JY, Lee JC, J. Am. Chem. Soc., 127(28), 9962 (2005)
  27. Wert MHB, Lambert M, Bourgoin JP, Brust M, Nano Lett., 2, 43 (2002)
  28. Reetz MT, Winter M, Dumpich G, Lohau J, Friedrichowski S, J. Am. Chem. Soc., 119(19), 4539 (1997)
  29. Corbierre MK, Beerens J, Lennox RB, Chem. Mater., 17, 5774 (2005)
  30. Clendenning SB, Aouba S, Rayat MS, Grozea D, Sorge JB, Brodersen PM, Sodhi RNS, Lu ZH, Yip CM, Freeman MR, Ruda HE, Manners I, Adv. Mater., 16(3), 215 (2004)
  31. Glass R, Arnold M, Blummel J, Kuller A, Moller M, Spatz JP, Adv. Funct. Mater., 13(7), 569 (2003)
  32. Yin DH, Horiuchi S, Morita M, Takahara A, Langmuir, 21(20), 9352 (2005)