Journal of Chemical Physics, Vol.103, No.10, 4157-4159, 1995
A Simple Method for Determining Approximate Static and Dynamic Vibrational Hyperpolarizabilities
A simple method is presented for calculating approximate static and dynamic vibrational hyperpolarizabilities. It involves determining electrical properties in the presence of a static field with and without geometry optimization. This method is readily applicable to all tenser components of a general polyatomic molecule.