Journal of Chemical Physics, Vol.105, No.23, 10424-10428, 1996
Control of Reactant Flow at the Boundary - Its Effect on the Onset of Nonequilibrium Macroscopic Structures in Chemical-Reactions
In a one-dimensional, two-component excitable chemical model system (the "Brusselator") we investigate the effects of controlling the flow of reactants at the boundary, on the stability of tho thermodynamical branch. The reflectivity of the boundary adjusts the external flux and acts as a control parameter, capable of enhancing or weakening the self-organizing processes lending to the appearance of temporal or spatial patterns.