화학공학소재연구정보센터
홈 로그인 로그아웃 연락처 사이트맵
Journal of Industrial and Engineering Chemistry, Vol.20, No.5, 2761-2768, September, 2014
DOI10.1016/j.jiec.2013.11.004  Export Citation
Experimental study of acetone removal by packed-bed dielectric barrier discharge reactor
Chenghang Zheng, Xinbo Zhu, Xiang Gao†, Lu Liu, Qianyun Chang, Zhongyang Luo, and Kefa Cen
  • State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, Zhejiang Province, PR China, Korea
E-mail:
In this study, a packed-bed dielectric barrier discharge (DBD) reactor was developed for acetone removal. The effects of packing materials were investigated in terms of discharge characteristics, removal efficiency and byproducts formation. The identification of organic byproducts was conducted. The results indicated the presence of packing materials enhanced the energy density and exhibited a positive effect on acetone removal, while high oxygen concentration inhibited the removal of acetone. The formations of byproducts were significantly reduced in the presence of packing materials. The degradation pathways and mechanisms were discussed, showing CH3 radicals played a crucial role in the acetone degradation process.
Keywords:Acetone;DBD;Packing materials;Decomposition reactions;Reaction pathways
  1. Holzer F, Roland U, Kopinke FD, Appl. Catal. B: Environ., 38(3), 163 (2002)
  2. Van Durme J, Dewulf J, Leys C, Van Langenhove H, Appl. Catal. B: Environ., 78(3-4), 324 (2008)
  3. Conti-Ramsden MG, Brown NW, Roberts EPL, Chem. Eng. J., 198, 130 (2012)
  4. Kim JB, Park JI, Kim HS, Yoo YJ, J. Ind. Eng. Chem., 18(1), 425 (2012)
  5. Das D, Gaur V, N. Verma, Carbon, 42, 2949 (2004)
  6. Lee JH, Nam W, Kang M, Han GY, Yoon KJ, Kim MS, Ogino K, Miyata S, Choung SJ, Appl. Catal. A: Gen., 244(1), 49 (2003)
  7. Kwon SH, Cho DC, J. Ind. Eng. Chem., 15(1), 129 (2009)
  8. Obradovic BM, Sretenovic GB, Kuraica MM, J. Hazard. Mater., 185(2-3), 1280 (2011)
  9. Mok YS, J. Ind. Eng. Chem., 11(6), 826 (2005)
  10. Pei MX, Lin H, Shangguan WF, Huang Z, Journal of Environmental Sciences-China, 17, 220 (2005)
  11. Chen HL, Lee HM, Chen SH, Chang MB, Ind. Eng. Chem. Res., 47(7), 2122 (2008)
  12. Bibinov N, Rajasekaran P, Mertmann P, Wandke D, Viol W, Awakowicz P, Laskovski A (Eds.), Basics and Biomedical Applications of Dielectric Barrier Discharge (DBD), 1st ed., InTech, Rijeka, pp. 123-150. (2011)
  13. Malik MA, Minamitani Y, Schoenbach KH, IEEE Transactions on Plasma Science, 33, 50 (2005)
  14. Magureanu M, Mandache NB, Parvulescu VI, Subrahmanyam C, Renken A, Kiwi-Minsker L, Appl. Catal. B: Environ., 74(3-4), 270 (2007)
  15. Callen MS, de la Cruz MT, Marinov S, Murillo R, Stefanova M, Mastral AM, Fuel Process. Technol., 88(3), 251 (2007)
  16. Harling AM, Demidyuk V, Fischer SJ, Whitehead JC, Appl. Catal. B: Environ., 82(3-4), 180 (2008)
  17. Ayrault C, Barrault J, Blin-Simiand N, Jorand F, Pasquiers S, Rousseau A, Tatibouet JM, Catal. Today, 89(1-2), 75 (2004)
  18. Li D, Zhang D, Wu Y, Li J, Li GF, Plasma Science & Technology, 10, 94 (2008)
  19. Han SB, Oda T, Ono R, IEEE Transactions on Industry Applications, 41, 1343 (2005)
  20. Lyulyukin MN, Besov AS, Vorontsov AV, Plasma Chem. Plasma Process., 31(1), 23 (2011)
  21. Lyulyukin MN, Besov AS, Vorontsov AV, Ind. Eng. Chem. Res., 52(17), 5842 (2013)
  22. Chang CL, Lin TS, Plasma Chem. Plasma Process., 25(3), 227 (2005)
  23. Holzer F, Kopinke FD, Roland U, Plasma Chem. Plasma Process., 25(6), 595 (2005)
  24. Takaki K, Shimizu M, Mukaigawa S, Fujiwara T, IEEE Transactions on Plasma Science, 32, 32 (2004)
  25. Liang WJ, Fang HP, Li J, Zheng F, Li JX, Jin YQ, Journal of Electrostatics, 69, 206 (2011)
  26. Vandenbroucke AM, Morent R, De Geyter N, Leys C, J. Hazard. Mater., 195, 30 (2011)
  27. Tu X, Gallon HJ, Whitehead JC, IEEE Transactions on Plasma Science, 39, 2172 (2011)
  28. Fridman A, Plasma Chemistry, 1st ed., Cambridge University Press, Cambridge (2008)
  29. Tu X, Gallon HJ, Whitehead JC, Journal of Physics D: Applied Physics, 44, 482003 (2011)
  30. Chen HL, Lee HM, Chen SH, Chao Y, Chang MB, Appl. Catal. B: Environ., 85(1-2), 1 (2008)
  31. Ding HX, Zhu AM, Yang XF, Li CH, Xu Y, Journal of Physics D: Applied Physics, 38, 4160 (2005)
  32. Kim HH, Ogata A, Futamura S, Appl. Catal. B: Environ., 79(4), 356 (2008)
  33. Lee HM, Chang MB, Plasma Chem. Plasma Process., 21(3), 329 (2001)
  34. Mok YS, Lee SB, Oh JH, Ra KS, Sung BH, Plasma Chem. Plasma Process., 28(6), 663 (2008)
  35. Wang H, Li D, Wu Y, Li J, Li G, Journal of Electrostatics, 67, 547 (2009)
  36. Magne L, Blin-Simiand N, Gadonna K, Jeanney P, Jorand F, Pasquiers S, Postel C, European Physical Journal: Applied Physics, 47, 22816 (2009)
  37. Futamura S, Yamamoto T, IEEE Transactions on Industry Applications, 33, 447 (1997)
  38. Blin-Simiand N, Jorand F, Magne L, Pasquiers S, Postel C, Vacher JR, Plasma Chem. Plasma Process., 28(4), 429 (2008)
  39. Machala Z, Hensel K, Marode E, in: Proceedings of CAPPSA (2005)
  40. McAdams R, Beech P, Shawcross JT, Plasma Chem. Plasma Process., 28(2), 159 (2008)
  41. van Durme J, Dewulf J, Sysmans W, Leys C, van Langenhove H, Chemosphere, 68, 1821 (2007)
  42. Ozensoy E, Herling D, Szanyi J, Catalysis Today, 136, 46 (2008)
  43. Huang HB, Ye DQ, Leung DYC, Feng FD, Guan XJ, J. Mol. Catal. A-Chem., 336(1-2), 87 (2011)
  44. Alzueta MU, Serinyel Z, Simmie JM, Curran HJ, Energy Fuels, 24, 1511 (1520)
  45. Sun WT, Uddi M, Won SH, Ombrello T, Carter C, Ju YG, Combust. Flame, 159(1), 221 (2012)