PTC (positive temperature coefficient) material is a kind of thermo-sensitive material. In this study, a series of novel PTC materials adapted to thermal control of electron devices are prepared. By adding different low-melting-point blend matrixes into GP (graphite powder)/LDPE (low density polyethylene) composite, the Curie temperatures are adjusted to 9 degrees C, 25 degrees C, 34 C and 41 degrees C, and the resistance-temperature coefficients are enhanced to 1.57/degrees C-2.15/degrees C. These PTC materials remain solid in the temperature region of PTC effect, which makes it possible to be used as heating element to achieve adaptive temperature control. In addition, the adaptive thermal control performances of this kind of materials are investigated both experimentally and theoretically. The result shows that the adaptive effect becomes more significant while the resistance-temperature coefficient increases. A critical heating power defined as the initial heating power which makes the equilibrium temperature reach terminal temperature is presented. The adaptive temperature control will be effective only if the initial power is below this value. The critical heating power is determined by the Curie temperature and resistance-temperature coefficient of PTC materials, and a higher Curie temperature or resistance-temperature coefficient will lead to a larger critical heating power. (C) 2014 Elsevier Ltd. All rights reserved.