Application of Fe0 aggregate in ultrasound enhanced advanced Fenton process for decolorization of methylene blue

Chih-Huang Weng; Vinson Huang

Journal of Industrial and Engineering Chemistry, Vol.28, 153-160, August, 2015

DOI10.1016/j.jiec.2015.02.010 Export Citation

Application of Fe0 aggregate in ultrasound enhanced advanced Fenton process for decolorization of methylene blue

Chih-Huang Weng^†, and Vinson Huang

Department of Civil and Ecological Engineering, I-Shou University, Da-Shu District, Kaohsiung 84001, Taiwan

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A successful decolorization of methylene blue (MB) was achieved through advanced Fenton’s process (AFP) coupled with sonolysis (sono-AFP) using zero-valent iron (Fe0) aggregate as a catalyst. The decolorization was dependent on the pH, Fe0, H2O2 doses, and acoustic power. Fe0 aggregate was reusable. A modified pseudo-first order equation was developed to describe the decolorization kinetics. To save electricity, short ultrasound irradiation was applied to the system. MB was completely degraded in the sono-AFP under optimized condition. The decolorization was obviously inhibited by the presence of Cl-, but it was unaffected by the presence of H2CO3, H2PO4-, ClO4-, NO3-, and SO4 2-

Keywords:Advanced Fenton process;Cationic dye;Color removal;Fe0 aggregate;Sonolysis

[References]

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[Referenced By]

[1] Findik S, Gunduz G, Ultrason. Sonochem., 14, 157 (2007)

[2] Weng CH, Lin YT, Liu N, Yang HY, Color. Technol., 130, 133 (2014)

[3] Karatas M, Argun YA, Argun ME, J. Ind. Eng. Chem., 18(3), 1058 (2012)

[4] Pukdee-Asa M, Su CC, Ratanatamskul C, Lu MC, Color. Technol., 128, 28 (2011)

[5] Liang J, Komarov S, Hayashi N, Kasai E, Ultrason. Sonochem., 14, 201 (2007)

[6] Segura Y, Martinez F, Meleroa JA, Molina R, Chand R, Bremner DH, Appl. Catal. B: Environ., 113-114, 100 (2012)

[7] Weng CH, Lin YT, Chang CK, Liu N, Ultrason. Sonochem., 20, 970 (2013)

[8] Grcic I, Papic S, Zizek K, Koprivanac N, Chem. Eng. J., 195-196, 77 (2012)

[9] Nidheesh PV, Gandhimathi R, Desalination, 299, 1 (2012)

[10] Bremner DH, Carlo SD, Chakinala AG, Cravotto G, Ultrason. Sonochem., 15, 416 (2008)

[11] Iglesias O, de Dios MAF, Tavares T, Sanroman MA, Pazos M, J. Ind. Eng. Chem., http://dx.doi.org/10.1016/j.jiec.2014.12.044. (2015)

[12] Pouran SR, Aziz ARA, Daud WMAW, J. Ind. Eng. Chem., 21, 53 (2015)

[13] Khataee A, Salahpour F, Fathinia M, Seyyedi B, Vahid B, J. Ind. Eng. Chem., (In press), http://dx.doi.org/10.1016/j.jiec.2014.11.024. (2014)

[14] Kim JR, Kan E, J. Ind. Eng. Chem., 21, 644 (2015)

[15] Yue L, Wang K, Guo J, Yang J, Luo X, Lian J, Wang L, J. Ind. Eng. Chem., 20(2), 725 (2014)

[16] Li JT, Song YL, Environ. Prog. Sustainable Energy, 29, 101 (2010)

[17] Chen B, Wang X, Wang C, Jiang W, Li S, Ultrason. Sonochem., 18, 1091 (2011)

[18] Sahinkaya S, J. Ind. Eng. Chem., 19(2), 601 (2013)

[19] Thiruverikatachari R, Vigneswaran S, Naidu R, J. Ind. Eng. Chem., 14(2), 145 (2008)

[20] Wilkin RT, Su C, Ford RG, Paul CJ, Environ. Sci. Technol., 39, 4599 (2005)

[21] Weng CH, Lin YT, Lin TY, Kao CM, J. Hazard. Mater., 149(2), 292 (2007)

[22] APHA, AWWA, WEF, Standard Methods for the Examination of Water and Wastewater, 22nd ed., American Public Health Association, Washington, DC, 2012.

[23] Buxton GV, Greenstock CL, Helman WP, J. Phys. Chem. Ref Data, 17, 513 (1998)

[24] Minero C, Pellizzari P, Maurino V, Pelizzetti E, Vione D, Appl. Catal. B: Environ., 77(3-4), 308 (2008)

[25] Roshani B, Leitner NKV, Chem. Eng. J., 168(2), 784 (2011)

[26] Ma HZ, Zhuo QF, Wang B, Chem. Eng. J., 155(1-2), 248 (2009)

[27] Ramirez JH, Costa CA, Madeira LM, Catal. Today, 107-108, 68 (2005)

[28] Wang X, Wang LG, Li JB, Qiu JJ, Cai C, Zhang H, Sep. Purif. Technol., 122, 41 (2014)