Molecular Crystals and Liquid Crystals, Vol.376, 141-146, 2002
Optical conductivity for possible ground states of dimerized two-band Pd(dmit)(2) salts
We have studied the optical conductivity for possible ground states of Pd(dmit)(2) salts, exactly diagonalizing a two-band Hubbard model for a dimer. Our results reproduce dominant peaks of the optical spectra measured by Tajima et al. and confirm their argument from the strong-coupling viewpoint. Interaction strengths are estimated and used to study the stability of magnetic orders.
Keywords:Pd(dmit)(2);dimerization;two-band Hubbard model;exact diagonalization;optical conductivity;magnetic frustration