화학공학소재연구정보센터
Journal of Non-Newtonian Fluid Mechanics, Vol.230, 43-67, 2016
Predicting large experimental excess pressure drops for Boger fluids in contraction-expansion flow
More recent finite element/volume studies on pressure-drops in contraction flows have introduced a variety of constitutive models to compare and contrast the competing influences of extensional viscosity, normal stress and shear-thinning. In this study, the ability of an extensional White-Metzner construction with FENE-CR model is explored to reflect enhanced excess pressure drops (epd) in axisymmetric 4:1:4 contraction-expansion flows. Solvent-fraction is taken as beta = 0.9, to mimic viscoelastic constant shear-viscosity Boger fluids. The experimental pressure-drop data of Rothstein & McKinley [1] has been quantitatively captured (in the initial pronounced rise with elasticity, and limiting plateau-patterns), via two modes of numerical prediction: (i) flow-rate Q-increase, and (ii) relaxation-time Xi-increase. Here, the former Q-increase mode, in line with experimental procedures, has proved the more effective, generating significantly larger enhanced-epd. This is accompanied with dramatically enhanced trends with De-incrementation in vortex-activity, and significantly larger extrema in NI, shear-stress and related extensional and shear velocity-gradient components. In contrast, the Xi-increase counterpart trends remain somewhat invariant to elasticity rise. Moreover, under Q-increase and with elasticity rise, a pattern of flow transition has been identified through three flow-phases in epd-data; (i) steady solutions for low to-moderate elasticity levels, (ii) Oscillatory solutions in the moderate elasticity regime (coinciding with Rothstein and McKinley [1] data), and (iii) finally solution divergence. New to this hybrid algorithmic formulation are - techniques in time discretisation, discrete treatment of pressure terms, compatible stress/velocity-gradient representation; handling ABS-correction in the constitutive equation, which provides consistent material-property prediction; and introducing purely-extensional velocity-gradient component specification at the shear-free centre flow-line through the velocity gradient (VGR) correction. (C) 2016 Elsevier B.V. All rights reserved.