In situ evaluation of corrosion damage using non-destructive electrochemical measurements-A case study

Sina S. Jamali; Yue Zhao; Zhiming Gao; Huijun Li; Ay Ching Hee

Journal of Industrial and Engineering Chemistry, Vol.43, 36-43, November, 2016

DOI10.1016/j.jiec.2016.07.045 Export Citation

In situ evaluation of corrosion damage using non-destructive electrochemical measurements-A case study

Sina S. Jamali^{1, 2}, Yue Zhao^{1, 2, †}, Zhiming Gao³, Huijun Li², and Ay Ching Hee²

¹ARC Research Hub for Australian Steel Manufacturing, Faculty of Engineering and Information Science, University of Wollongong, Wollongong, NSW 2522, Australia
²School of Mechanical, Materials, and Mechatronics Engineering, Faculty of Engineering and Information Sciences, University of Wollongong, Wollongong, NSW 2500, Australia
³School of Materials Science and Engineering, Tianjin University, Tianjin 300072, China

E-mail:

Field application of electrochemical measurements with a non-invasive electrode arrangement has been used for investigating corrosion damage and protectiveness of a paint coating on an artwork sculpture. For this field application solid state probes were designed and used in electrochemical impedance spectroscopy (EIS) and electrochemical noise measurement (ENM) to evaluate the level of corrosion protection afforded by the paint coating. Samples were also analyzed in laboratory using analytical techniques. Results of electrochemical measurements indicated poor protective properties of the paint coating while analytical examinations revealed an inhomogeneous structure of the coating and a highly porous structure of the oxide scale.

Keywords:In situ evaluation;Electrochemical impedance spectroscopy;Electrochemical noise measurement;Solid state electrode;Non-destructive measurement;Corrosion

[References]

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[1] Groysman A, in: Groysman A (Ed.), Corrosion in Systems for Storage & Transportation of Petroleum Products & Biofuels, Netherlands, Springer, 2014, pp. 187.

[2] Mickalonis JI, Tshishiku EM, Edgemon GL, Development of a Movable Electrochemical Noise Corrosion Probe for Nuclear Waste Tanks, technical report WSRC-MS-2001-00734, 2002.

[3] Townley DW, Duranceanu SJ, Wilson DF, Corrosion, NACE International, Houston, TX, 2002 paper no. 02328.

[4] Barr E, Pierrerd L, Greenfield A, NACE Corrosion, NACE International, Houston, Texas, 2001 paper no. 01288.

[5] Covino BS, Bullard SJ, Cramer SD, Holcomb GR, Ziomek-Moroz M, Cayard MS, Eden DC, Kane RD, Corrosion/2004, NACE International Houston, TX, New Orleans, LA, 2004.

[6] Ruedisueli RL, Murray JN, Corrosion 2004, New Orleans, LA, 2004, paper no. 04297.

[7] Murray JN, in: Bierwagen GP (Ed.), Organic Coatings for Corrosion Control, ACS Symposium Series, 1998, p. 10.

[8] Murray JN, Ruedisueli R, Corrosion 2005, NACE International, 2005 paper no. 05219.

[9] Angelini E, Grassini S, Parvis M, Zucchi F, Surf. Interface Anal., 44(8), 942 (2012)

[10] Corbellini S, Parvis M, Grassini S, IEEE Trans. Instrum. Meas., 61(5), 1193 (2012)

[11] Woodcock CP, Mills DJ, Singh HT, J. Corros. Sci. Eng., 8, 1 (2004)

[12] Mabbutt SJ, Mills DJ, Woodcock CP, Prog. Org. Coat., 59(3), 192 (2007)

[13] Toku, ACT Government, artsACT, http://www.arts.act.gov.au/arts-in-the-act/public-art/toku, (accessed 23.09.15).

[14] Mills DJ, Broster M, Razaq I, Prog. Org. Coat., 63(3), 267 (2008)

[15] Mills DJ, Jamali SS, Tobiszewski MT, Prog. Org. Coat., 74(2), 385 (2012)

[16] Jamali SS, Mills DJ, Woodcock CP, ECS Trans., 24(1), 115 (2010)

[17] Mills D, Picton P, Mularczyk L, Electrochim. Acta, 124, 199 (2014)

[18] Gelling VJ, Electrochemical impedance spectroscopy method and system, U.S. Patent. WO2007095573, 2007.

[19] Gelling VJ, Field Coating Measurement, http://www.ndsu.edu/faculty/vijohnst/research/electrochemical_methods/, (accessed 29.05.15).

[20] Ritter S, Huet F, Cottis RA, Mater. Sci., 63(4), 297 (2012)

[21] Jamali SS, Mills DJ, Sykes JM, Prog. Org. Coat., 77, 733 (2014)

[22] Skerry B, Eden D, Prog. Org. Coat., 19(April 1), 379 (1991)

[23] Bacon RC, Smith JJ, Rugg FM, Ind. Eng. Chem., 40(1), 161 (1948)

[24] Cottis RA, Turgoose S, Mendoza-Flores J, in: Kearns JR, Scully JR, Roberge PR, Reichert DL, Dawson JL (Eds.), Electrochemical Noise Measurement for Corrosion Applications, ASTM STP1277, American Socienty for Testing and Materials, 1996, pp. 93.

[25] Moongkhamklang P, Taylor S, Prog. Org. Coat., 46(4), 259 (2003)

[26] Taylor SR, Moongkhamklang P, Prog. Org. Coat., 54(3), 205 (2005)

[27] Jamali SS, Mills DJ, Prog. Org. Coat., 77(12), 2091 (2014)

[28] Ploeger R, Scalarone D, Chiantore O, J. Cult. Herit., 9, 412 (2008)