Journal of Physical Chemistry, Vol.99, No.18, 6789-6793, 1995
Optimal-Control of Electronic Excitation in Molecular Aggregates
We present a theoretical study on optimal control of the electronic excitation in molecular aggregates with disorder. The intermolecular interactions are evaluated under the local field approximation. Numerical calculations on optimal control of population inversion of a uniform molecular aggregate an presented. The effect of intermolecular interactions and disorder upon the optimal field are examined.
Keywords:SIMULTANEOUS OMEGA-1;OMEGA-3 EXCITATION;MIRRORLESS OPTICAL BISTABILITY;UNIMOLECULAR REACTIONS;SELECTIVE EXCITATION;LASER-PULSES;SPECTROSCOPY;PHASE