We report predictions of the unpolarized vibrational absorption and vibrational circular dichroism spectra of 10 chiral molecules based on harmonic force fields calculated ab initio using density functional theory. The molecules are 1, oxirane (ethylene oxide)-trans-2,3-d(2); 2, methyloxirane (propylene oxide); 3, trans-2,3-dimethyloxirane; 4, trans-2,3-dimethyloxirane-2-d(1);5, trans-2,3-dimethyloxirane-trans-2,3-d(2); 6, methylthiirane (propylene sulfide); 7, trans-2, 3-dimethylthiirane; 8, trans-2,3-dimethylthiirane-trans-2,3-d(2); 9, cyclopropanet-trans-1,2-d(2); 10, cyclopropane-anti-1,2,3-d(3)-1-C-13. Large TZ2P basis sets are used to minimize basis set error. Three density functionals are employed : (1) the local spin density (LSDA) functional, (2) the Becke-Lee-Yang-Parr (BLYP) nonlocal functional, and (3) the Becke 3-Lee-Yang-Parr (B3LYP) hybrid functional. Predicted spectra are sensitive to the choice of density functional. Spectra predicted using the B3LYP functional are in the best agreement with experimental spectra while spectra predicted using the LSDA functional are in the worst agreement. Spectra predicted using the BLYP functional are more similar to those obtained using the B3LYP functional. We conclude that the relative accuracies of the functionals are B3LYP > BLYP much greater than LSDA.