Journal of Physical Chemistry A, Vol.102, No.23, 4310-4320, 1998
Laser control of atomic motion inside diatomic molecules
Globally optimal solution describing a phase conjugated field of Raman scattering on the resonant B <-- X transition of iodine I-2 is studied. Maximum optical coherence is found as a top eigenvalue problem. A reversibility theorem has been stated. This provides sufficient conditions for a tightly localized waveform and molecular hologram to exist. A noisy picosecond pulse has been computed to show how femtosecond polarization is regained at target time.
Keywords:INFRARED ABSORPTION-SPECTRUM;QUANTUM-MECHANICAL COMPUTERS;WAVE-PACKET EVOLUTION;PULSES;DYNAMICS;INTERFEROMETRY;SELECTIVITY;I2