A selection of experimental measurements for He-Ar, He-N-2, and He-Ne binary gas mixtures which were made with a spinning rotor gauge (SRG) are reported. All of the experiments were conducted in the slip regime. Theoretical results from a previous paper on the SRG are used to extract values of the viscosity and the velocity slip coefficient from the experimentally obtained data for each of the gas mixtures. The measured viscosities are in excellent agreement with existing literature values. Slip coefficients for binary gas mixtures have not previously been reported. An important issue here is whether the velocity slip coefficients for binary gas mixtures can be predicted accurately using separately measured tangential momentum accommodation coefficients. The calculation of slip coefficients from theory requires a knowledge of the accommodation coefficients of each constituent of the mixture. The dependence of these coefficients on the gas composition is not known and the simplest assumption is to regard them as being independent of the composition. The slip coefficients computed in conjunction with this work use this simple assumption in a theoretical expression for the slips. These computations led to reasonable agreement of the theoretical results with our data for the He-Ne mixture. Agreement in the cases of the He-Ar and He-N2 mixtures, however, was less than satisfactory.