Drying with solar-heated air is satisfactory so long as the sun is shining.; To continue this process through the night-time and periods of cloud cover, it is necessary to either store some of this energy in a thermal mass or incorporate desiccants within the drying system. This paper reports the results from studies undertaken to develop three low cost, solar regenerative clay-CaCl2 based solid desiccant materials; establish their moisture sorption and regeneration characteristics; assess their performance when compared with commercial desiccants; and integrate these within a low cost solar drying system for small-scale village-based crop drying. The moisture sorption and desorption performance of the desiccants were characterised in a Fison Environmental Cabinet at conditions of 85% (:RH) and 25 degrees C for 120 h for moisture sorption and 50 degrees C and 20% (RH) for 8 h for regeneration. These conditions were representative of the environmental conditions monitored in the solar drying system. The bentonite-CaCl2 (type 1) desiccant gave a maximum moisture sorption of 45% dry weight basis (dwb) while bentonite-CaCl2 (type 2) and kaolinite-CaCl2 (type 3) solid desiccants each gave moisture sorption values of 30% (dwb). It was concluded from the moisture sorption and regeneration characteristics that their application in solar crop drying and air dehumidification is highly useful due to their low regeneration temperatures, sub 100 degrees C,