The region around the minimum of the potential-energy curve of Cr-2 has been calculated at the multireference configuration interaction (CI) level including almost 1.3 billion configurations in the CI calculation. The computational techniques as implemented on massively parallel computers which enabled this calculation are described. The calculated results are R-e = 1.72 Angstrom, D-e = 1.09 eV, and omega(e) = 338.7 cm(-1) as compared to experimental values of R-e = 1.679 Angstrom, D-e = 1.50 +/- 0.05 eV, and omega(e) = 452.34(Delta G(1/2)) cm(-1). The error of 0.4 eV in the dissociation energy can be attributed to relativistic effects following other authors (0.2 eV) and the need for higher angular momentum basis functions in the one-particle set (0.2 eV).