The principal objective of the present study is to develop suitable models to predict aromaticity of coals on the basis of atomic ratios of the H/C, O/C O/H, and weight percentage volatile matter (V.M.) in coals. Based on dry mineral matter free (dmmf) basis, aromaticity (fa) of coal is computed through the following expressions:fa(1) = 1.202913 - 0.01216* V.M., (2)fa(2) = 1.36396 - 0.53715*O/C - 0.7846*H/C, (3)fa(3) = 1.365615 - 0.51187*O/C - 0.02108*O/H - 0.78645*H/C, (4)fa(4) =174.4405 + 621.6823*O/C - 856.495*O/H - 629.617*H/C + 9.133897*V.M. (5)The absolute average % error of estimate and correlation coefficients of the developed models (Equations (2), (3) (4), and (5)) were found to be 7.48.0.91: 6.23. 0.92; 6.24, 0.92; and 6.23, 0.92 on (dmmf) basis, respectively.