화학공학소재연구정보센터
Journal of Industrial and Engineering Chemistry, Vol.15, No.6, 865-869, November, 2009
Leaching kinetics of calcined magnesite in acetic acid solutions
E-mail:
The leaching kinetics of calcined magnesite by using acetic acid solutions was investigated in a batch reactor by using the parameters such as temperature, acid concentration and particle size. The experimental results were successfully correlated by linear regression using Statistica Package Program. Dissolution curves were evaluated in order to test shrinking core models for fluid.solid systems. It was concluded that the leaching of calcined magnesite was controlled by chemical reaction. In addition, the fact that leaching was controlled by the chemical reaction was also supported with the relationship between the reaction rate constant and the particle radius. The apparent activation energy of dissolution process was found as 34.60 kJ mol^(-1).
  1. Demirkiran N, Hydrometallurgy, 95, 198 (2009)
  2. Hursit M, Lacin O, Sarac H, J. Taiwan Inst. Chem. Eng., 40, 6 (2009)
  3. Ekmekyapar A, Demirkiran N, Kunkul A, Chem. Eng. Res. Des., 86(9A), 1011 (2008)
  4. Bakan F, Lacin O, Bayrak B, Sarac H, Int. J. Miner. Process., 80, 27 (2006)
  5. Bayrak B, Lacin O, Bakan F, Sarac H, Chem. Eng. J., 117(2), 109 (2006)
  6. Kralj AK, J. Ind. Eng. Chem., 13(4), 631 (2007)
  7. Lee KW, Yu JX, Mei JH, Yan L, Kim YW, Chung KW, J. Ind. Eng. Chem., 13(5), 799 (2007)
  8. Tzeferis PG, Agatzini-Leonardou S, Hydrometallurgy, 36, 345 (1994)
  9. Lacin O, Donmez B, Demir F, Int. J. Miner. Process., 75, 91 (2005)
  10. Demir F, Donmez B, Colak S, J. Chem. Eng. Jpn., 36(6), 683 (2003)
  11. Demirkiran N, Chem. Eng. J., 141(1-3), 180 (2008)
  12. ERSAHAN H, EKMEKYAPAR A, SEVIM F, Int. J. Miner. Process., 42(1), 121 (1994)
  13. Demir F, Donmez B, Okur H, Sevim F, Chem. Eng. Res. Des., 81(6), 618 (2003)
  14. Hawley GG, The Condensed Chemical Dictionary, 9th ed., Van Nostarnd Reinhold Company, New York, 1977, p. 528.
  15. Glaser V, Vidensky J, Kuzela M, Collect. Czech. Chem. Commun., 53, 1711 (1988)
  16. Economou ED, Vaimakis TC, Papamichael EM, J. Colloid Interface Sci., 201(2), 164 (1998)
  17. Fredd CN, Fogler HS, Chem. Eng. Sci., 53(22), 3863 (1998)
  18. Demir F, Lacin O, Donmez B, Ind. Eng. Chem. Res., 45(4), 1307 (2006)
  19. Furmann NH, Standard Methods of Chemical Analysis, 6th ed., D. Van. Nastrand Company, New Jersey, 1963.
  20. Gulensoy H, Kompleksometrik Titrasyonlar ve Kompleksometrinin Temelleri, Fatih Yayınevi, I˙stanbul, Turkey, 1974.
  21. Marinovic V, Despic AR, J. Electroanal. Chem., 431(1), 127 (1997)
  22. Levenspiel O, Chemical Reaction Engineering, 2nd ed., John Wiley and Sons Inc., New York, 1972.