화학공학소재연구정보센터
Journal of Physical Chemistry B, Vol.113, No.17, 5897-5904, 2009
Width of Phonon Sidebands in the Brownian Oscillator Model
The line width dependence of zero-phonon lines and phonon sidebands oil temperature, bath dissipation, and electron-phonon coupling is studied for an underdamped Brownian oscillator model with an Ohmic dissipative bath. Factors determining the line widths vary from the zero-phonon lines to the phonon sidebands. The control-parameter space of line broadening has been mapped out, revealing that the line widths of the zero-phonon lines and phonon sidebands are linearly dependent on both the temperature and the Huang-Rhys factor. It is also found that the dependence of the line widths oil the bath damping factor is linear for the zero-phonon lines and quadratic for the phonon sidebands.