Quantum phenomena of interest in connection with applications to computation and communication often involve generating specific transfers between eigenstates, and their linear superpositions. For some quantum systems, such as spin systems, the quantum evolution equation (the Schrodinger equation) is finite-dimensional and old results on controllability of systems defined on on Lie groups and quotient spaces provide most of what is needed insofar as controllability of non-dissipative systems is concerned. However, in an infinite-dimensional setting, controlling the evolution of quantum systems often presents difficulties, both conceptual and technical. In this paper we present a systematic approach to a class of such problems for which it is possible to avoid some of the technical issues. In particular, we analyze controllability for infinite-dimensional bilinear systems under assumptions that make controllability possible using trajectories lying in a nested family of pre-defined subspaces. This result, which we call the Finite Controllability Theorem, provides a set of sufficient conditions for controllability in an infinite-dimensional setting. We consider specific physical systems that are of interest for quantum computing, and provide insights into the types of quantum operations (gates) that may be developed.