화학공학소재연구정보센터
학회 한국공업화학회
학술대회 2022년 봄 (05/11 ~ 05/13, 제주국제컨벤션센터(ICC JEJU))
권호 26권 1호
발표분야 포스터-환경·에너지
제목 N-doped graphene oxide enfolded reduced titania for highly stable andselective gas-phase photocatalytic CO2 reduction into CH4
초록 A desire for renewable alternatives to fossil fuelscan be achieved by utilizing CO2, H2O, and solar energyto generate solar fuels. Herein, N-doped graphene oxide enfolded reducedtitania (NGO-RT) composite was demonstrated for photocatalytic CO2reduction into CH4. Further, the Pt NPs were deposited on NGO-RTthat increases the catalytic performance towards CH4 formation. Theoptimized Pt1.0%-NGO-RT catalyst displayed a selective visible-lightCO2 reduction into CH4 using a flow reactor system with ≈12 and ≈2 times higheractivity than pristine RT and NGO-RT, respectively. The catalyst demonstratedlong-term stability over 35 h. The improved catalytic performance can beattributed to RT’s downward band bending at the NGO-RT interface, whereelectron transfer from RT to NGO decreases the charge recombination.

저자 Chaitanya B. Hiragond, 인수일
소속 DGIST
키워드 Reduced titania; N-doped GO; Photocatalysis CO2 reduction; Flow-reactor system
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