학회 | 한국공업화학회 |
학술대회 | 2022년 봄 (05/11 ~ 05/13, 제주국제컨벤션센터(ICC JEJU)) |
권호 | 26권 1호 |
발표분야 | 포스터-환경·에너지 |
제목 | N-doped graphene oxide enfolded reduced titania for highly stable andselective gas-phase photocatalytic CO2 reduction into CH4 |
초록 | A desire for renewable alternatives to fossil fuelscan be achieved by utilizing CO2, H2O, and solar energyto generate solar fuels. Herein, N-doped graphene oxide enfolded reducedtitania (NGO-RT) composite was demonstrated for photocatalytic CO2reduction into CH4. Further, the Pt NPs were deposited on NGO-RTthat increases the catalytic performance towards CH4 formation. Theoptimized Pt1.0%-NGO-RT catalyst displayed a selective visible-lightCO2 reduction into CH4 using a flow reactor system with ≈12 and ≈2 times higheractivity than pristine RT and NGO-RT, respectively. The catalyst demonstratedlong-term stability over 35 h. The improved catalytic performance can beattributed to RT’s downward band bending at the NGO-RT interface, whereelectron transfer from RT to NGO decreases the charge recombination. |
저자 | Chaitanya B. Hiragond, 인수일 |
소속 | DGIST |
키워드 | Reduced titania; N-doped GO; Photocatalysis CO2 reduction; Flow-reactor system |