화학공학소재연구정보센터
Journal of Industrial and Engineering Chemistry, Vol.23, 316-320, March, 2015
Effect of sulfonated poly(arylene ether sulfone) binder on the performance of polymer electrolyte membrane fuel cells
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To achieve good interfacial compatibility between the membrane and electrode, structure modification of sulfonated poly(arylene ether sulfone) (SPAES) was successfully done for use as an electrode binder for polymer electrolyte membrane fuel cells. A new activation method for hydrocarbon membrane-electrode assembly (MEA) with a hydrocarbon binder was developed using a voltage cycle instead of applying a constant voltage, which is a standard activation method for MEA with a Nafion binder. To investigate the effect of the binder, two SPAES samples with different molecular weights were used for characterization, and the composition of the binder was also optimized.
  1. Arico AS, Srinivasan S, Antonucci V, Fuel Cells, 1, 133 (2001)
  2. Wasmus S, Kuver A, J. Electroanal. Chem., 461(1-2), 14 (1999)
  3. Hogarth MP, Hards GA, Platinum Met. Rev., 40, 150 (1996)
  4. Yoon KS, Lee JY, Kim TH, Yu DM, Seo DW, Hong SK, Hong YT, J. Ind. Eng. Chem., 20(4), 2310 (2014)
  5. Kim DJ, Hwang HY, Jung SB, Nam SY, J. Ind. Eng. Chem., 18(1), 556 (2012)
  6. Yu DM, Yoon K, Yoon YJ, Kim TH, Lee JY, Hong YT, Macromol. Chem. Phys., 213, 839 (2012)
  7. Peighambardoust SJ, Rowshanzamir S, Amjadi M, Int. J. Hydrog. Energy, 35(17), 9349 (2010)
  8. Yu DM, Yoon YJ, Kim TH, Lee JY, Hong YT, Solid State Ion., 233, 55 (2013)
  9. Bose S, Kuila T, Nguyen TXH, Kim NH, Lau K, Lee JH, Prog. Polym. Sci, 36, 813 (2011)
  10. Adjemian KT, Lee SJ, Srinivasan S, Benziger J, Bocarsly AB, J. Electrochem. Soc., 149(3), A256 (2002)
  11. Yang C, Srinivasan S, Bocarsly AB, Tulyani S, Benziger JB, J. Membr. Sci., 237(1-2), 145 (2004)
  12. Zhai YF, Zhang HM, Hu JW, Yi BL, J. Membr. Sci., 280(1-2), 148 (2006)
  13. Higashihara T, Matsumoto K, Ueda M, Polymer, 50(23), 5341 (2009)
  14. Li Q, He R, Jensen JO, Bjerrum NJ, Fuel Cells, 4, 147 (2004)
  15. Bonnet B, Jones DJ, Roziere J, Tchicaya L, Alberti G, Casciola M, Massinelli L, Bauer B, Peraio A, Ramunni E, J. New Mat. Electrochem. Syst., 3, 87 (2000)
  16. Nagarale RK, Shin W, Singh PK, Polym. Chem., 1, 388 (2010)
  17. Kerres J, Ullrich A, Meier F, Haring T, Solid State Ion., 125(1-4), 243 (1999)
  18. Ko H, Yu DM, Choi JH, Kim HJ, Hong YT, J. Membr. Sci., 390-391, 226 (2012)
  19. Hickner MA, Ghassemi H, Kim YS, Einsla BR, McGrath JE, Chem. Rev., 104(10), 4587 (2004)
  20. Wang F, Hickner M, Kim YS, Zawodzinski TA, McGrath JE, J. Membr. Sci., 197(1-2), 231 (2002)
  21. Hong YT, Lee CH, Park HNS, Min KA, Kim HJ, Nam SY, Lee YM, J. Power Sources, 175(2), 724 (2008)
  22. Wang F, Hickner M, Ji Q, Harrison W, Mecham J, Zawodzinski TA, McGrath JE, Macromol. Symp., 175, 387 (2001)
  23. Peron J, Shi Z, Holdcroft S, Energy Environ. Sci., 4, 1575 (2011)
  24. Jung HY, Cho KY, Sung KA, Kim WK, Kurkuri M, Park JK, Electrochim. Acta, 52(15), 4916 (2007)
  25. Kim YS, Chlistunoff J, Pivovar BS, DOE hydrogen program review, May 16 (2006), Washington DC, USA.
  26. Park JY, Kim TH, Kim HJ, Choi JH, Hong YT, Int. J. Hydrog. Energy, 37(3), 2603 (2012)
  27. Park YJ, Yu DK, Ahn JH, Choi JH, Hong YT, Macromol. Res., 20(2), 168 (2012)
  28. Kim YS, Einsla B, Sankir M, Harrison W, Pivovar BS, Polymer, 47(11), 4026 (2006)
  29. Xie JA, Xu F, Wood DL, More KL, Zawodzinski TA, Smith WH, Electrochim. Acta, 55(24), 7404 (2010)
  30. Jung HY, Cho KY, Sung KA, Kim WK, Park JK, J. Power Sources, 163(1), 56 (2006)