화학공학소재연구정보센터
Journal of Crystal Growth, Vol.211, No.1-4, 86-92, 2000
H-dependent magnetic domain structures in La0.67Sr0.33MnO3 thin films
Maze- and bubble-like magnetic domain structures hale been observed under ambient conditions in La0.67Sr0.33MnO3 (LSMO) films by magnetic force microscopy (MFM) for films grown on a compressive (LaAlO3) lattice-mismatched substrate. The substrate-induced stress in this soft magnetic material appears to be a necessary but not sufficient condition For the appearance of these structures. i.e. no magnetic structure has been seen for other films grown under similar conditions on the same substrate with similar distortions to the unit cell. In this study, in order to understand the stability of these structures, we have examined two films grown at 750 degrees C and three films grown at 800 C by pulsed-laser deposition by scanning tunneling and magnetic force microscopy to obtain microstructure and domain structures as a function of in-plane magnetic field strength. The latter films consisted of pitted coalesced layers with some surface 3D growth Although the films were nominally grown under the same conditions, there were subtle differences in the domain structure, wall spacing, the latter due in part to differences in film thickness, and response to an applied in-plane magnetic field. As the held was increased. the maze-libe structures became stripe domains with reduced out-of-plane magnetization and decreased wall spacing, consistent with parallel rather than antiparallel alignment of in-plane spin polarization. After removal of the field, the stripe domains remained but the wall spacing and z polarization component returned to the original value. For one 800 degrees C film the field required for changes in and disappearance of the domains paralleled the slope in the field-dependent magnetization. In contrast, the magnetic structure for one film with a thin insulating cap layer was reversible, suggesting that the walls were pinned by the cap. Published by Elsevier Science B.V.