화학공학소재연구정보센터
홈 로그인 로그아웃 연락처 사이트맵
Journal of Industrial and Engineering Chemistry, Vol.49, 1-25, May, 2017
DOI10.1016/j.jiec.2016.12.003  Export Citation
Hydrogen production: Perspectives, separation with special emphasis on kinetics of WGS reaction: A state-of-the-art review
Samrand Saeidi1, 2, Farhad Fazlollahi3, Sara Najari4, Davood Iranshahi2, Jiri Jarmir Klemes5, †, and Larry L. Baxter6
  • 1Department of Wood and Paper Science, Research Institute of Forests and Rangelands, Agricultural Research, Education and Extension Organization (AREEO), Tehran, Iran
  • 2School of Chemical Engineering, Amirkabir University of Technology (Tehran Polytechnic), No. 424, Hafez Avenue, 15914 Tehran, Iran
  • 3School of Chemical Engineering, Purdue University, 480 Stadium Mall Dr., West Lafayette, IN 47906, USA
  • 4Department of Chemical Engineering, Tarbiat Modares University, Tehran 14115-114, Iran
  • 5Pázmány Péter Catholic University, 1088 Budapest, Szentkirályi utca 28, Hungary
  • 6Chemical Engineering Department, Brigham Young University, Provo, UT 84602, USA
E-mail:
Fossil fuel depletion, global warming, energy security, and climate change spur interest in commercial and environmentally friendly alternative fuels. Palladium-based catalytic membrane technology currently produces ultrapure hydrogen from fossil fuels. Palladium exhibits high permeability, selectivity for hydrogen, and good surface properties. Properties of some palladium alloys enable the industrial production of hydrogen. Reaction rates and conversion depend on several parameters. This document reviews kinetic expressions for the water.gas shift (WGS) reactions and WGS combined with Fischer. Tropsch synthesis (WGS.FTS) reactions at high and low temperatures along with the details of the catalysts and operating conditions. The discussion includes mathematical reactor modeling.
Keywords:Water.gas shift reaction;Pd-alloy membrane;Reaction kinetic models;Membrane reactor;Hydrogen production
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